| Record of the Year |
"A Taste of Honey", Herb Alpert and the Tijuana Brass |
| Album of the Year |
September of My Years, Frank Sinatra (Reprise) |
| Song of the Year |
"The Shadow of Your Smile” (Love Theme From The Sandpiper), Paul Francis Webster and Johnny Mandel, songwriters |
| Best New Artist |
Tom Jones |
| Most Promising New Recording Artist |
Peter Serkin, pianist |
| Best Vocal Performance, Male |
"It Was a Very Good Year", Frank Sinatra |
Best Vocal Performance, Female
 Barbra Streisand
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My Name Is Barbra, Barbra Streisand |
| Best Performance By a Vocal Group |
We Dig Mancini, Anita Kerr Singers |
| Best Performance By a Chorus |
Anyone for Mozart?, Swingle Singers |
| Best Contemporary (Rock and Roll) Single |
"King of the Road", Roger Miller |
| Best Contemporary (Rock and Roll) Vocal Performance, Male |
"King of the Road", Roger Miller |
| Best Contemporary (Rock and Roll) Vocal Performance, Female |
"I Know a Place", Petula Clark |
| Best Contemporary (Rock and Roll) Performance Group (Vocal or Instrumental) |
"Flowers on the Wall", Statler Brothers |
| Best Rhythm and Blues Recording |
"Papa's Got a Brand New Bag", James Brown (King) |
| Best Instrumental Jazz Performance, Small Group or Soloist With Small Group |
The "In” Crowd, Ramsey Lewis Trio |
| Best Instrumental Jazz Performance, Large Group or Soloist With Large Group |
Ellington '66, Duke Ellington Orchestra |
| Best Original Jazz Composition |
Jazz Suite on the Mass Texts, Lalo Shifrin, composer |
| Best Country and Western Single |
"King of the Road", Roger Miller |
| Best Country and Western Album |
The Return of Roger Miller, Roger Miller (Smash) |
| Best Country and Western Song |
"King of the Road", Roger Miller, songwriter |
| Best Country and Western Vocal Performance, Male |
"King of the Road", Roger Miller |
| Best Country and Western Vocal Performance, Female |
"Queen of the House", Jody Miller |
| Best New Country and Western Artist |
Statler Brothers |
| Best Gospel or Other Religious Recording (Musical) |
Southland Favorites, George Beverly Shea and the Anita Kerr Quartet (RCA) |
| Best Folk Recording |
An Evening With Belafonte/Makeba, Harry Belafonte and Miriam Makeba (RCA) |
| Best Instrumental Arrangement |
"A Taste of Honey", Herb Alpert, arranger |
| Best Arrangement Accompanying a Vocalist or Instrumentalist |
"It Was a Very Good Year", Gordon Jenkins, arranger |
| Best Instrumental Performance, Non-Jazz |
"A Taste of Honey", Herb Alpert and the Tijuana Brass |
| Best Score From an Original Show Album |
On a Clear Day, Alan Lerner and Burton Lane (RCA) |
| Best Original Score Written for a Motion Picture or Television Show |
The Sandpiper, Johnny Mandel, composer (Mercury) |
| Album of the Year, Classical |
Horowitz at Carnegie Hall, An Historic Return, Vladimir Horowitz (Columbia) |
| Best Classical Performance, Orchestra |
Ives, Symphony No. 4, Leopold Stokowski conducting American Symphony Orchestra |
| Best Classical Chamber Music Performance, Instrumental or Vocal |
Bartók, The Six String Quartets, Juilliard String Quartet |
| Best Classical Performance, Instrumental Soloist(s) (With Orchestra) |
Beethoven, Concerto No. 4 in G Major for Piano and Orchestra, Artur Rubinstein; Erich Leinsdorf conducting Boston Symphony |
| Best Classical Performance, Instrumental Soloist (Without Orchestra) |
Horowitz at Carnegie Hall, An Historic Return, Vladimir Horowitz |
| Best Opera Recording |
Berg, Wozzeck, Karl Bohm conducting Orchestra of German Opera, Berlin; solos: Fisher-Dieskau, Lear and Wunderlich (Deutsche Grammophon) |
| Best Classical Choral Performance (Other Than Opera) |
Stravinsky, Symphony of Psalms; Poulenc, Gloria, Robert Shaw conducting Robert Shaw Chorale and RCA Victor Symphony Orchestra |
| Best Classical Vocal Performance, With or Without Orchestra |
Strauss, Salome ("Dance of the Seven Veils", Interlude, Final Scene); The Egyptian Helen (Awakening Scene), Leontyne Price |
| Best Composition By a Contemporary Classical Composer |
Symphony No. 4, Charles Ives, composer |
| Best Comedy Performance |
Why Is There Air?, Bill Cosby |
| Best Spoken Word or Drama Recording |
John F. Kennedy: As We Remember Him (Columbia) |
| Best Recording for Children |
Dr. Seuss Presents "Fox in Sox” and "Green Eggs and Ham", Marvin Miller (RCA) |
| Best Album Cover, Graphic Arts |
Bartók, Concerto No. 2 for Violin; Stravinsky, Concerto for Violin, James Alexander, graphic artist; George Estes, art director (RCA) |
| Best Album Cover, Photography |
Jazz Suite on the Mass Texts, Ken Whitmore, photographer; Bob Jones, art director (RCA) |
| Best Album Notes |
September of My Years, Stan Cornyn, annotator (Reprise) |
