| Record of the Year |
"Mrs. Robinson", Simon and Garfunkel |
| Album of the Year |
By the Time I Get to Phoenix, Glen Campbell (Capitol) |
| Song of the Year |
"Little Green Apples", Bobby Russell, songwriter |
| Best New Artist of 1968 |
José Feliciano |
| Best Contemporary Pop Vocal Performance, Male |
"Light My Fire", José Feliciano |
| Best Contemporary Pop Vocal Performance, Female |
"Do You Know the Way to San Jose", Dionne Warwick |
| Best Contemporary Pop Vocal Performance, Duo or Group |
"Mrs. Robinson", Simon and Garfunkel |
| Best Contemporary Pop Performance, Chorus |
"Mission Impossible/Norwegian Wood (medley), Alan Copeland Singers |
| Best Contemporary Pop Performance, Instrumental |
"Classical Gas", Mason Williams |
| Best Rhythm and Blues Song |
(Sittin' On) "The Dock of the Bay", Otis Redding and Steve Cropper, songwriters |
| Best Rhythm and Blues Vocal Performance, Male |
(Sittin' On) "The Dock of the Bay", Otis Redding |
| Best Rhythm and Blues Vocal Performance, Female |
"Chain of Fools", Aretha Franklin |
| Best Rhythm and Blues Performance By a Duo or Group, Vocal or Instrumental |
"Cloud Nine", The Temptations |
| Best Instrumental Jazz Performance, Small Group or Soloist With Small Group |
Bill Evans at the Montreux Jazz Festival, Bill Evans Trio |
| Best Instrumental Jazz Performance, Large Group or Soloist With Large Group |
"And His Mother Called Him Bill", Duke Ellington |
| Best Country Song |
"Little Green Apples", Bobby Russell, songwriter |
| Best Country Vocal Performance, Male |
"Folsom Prison Blues", Johnny Cash |
| Best Country Vocal Performance, Female |
"Harper Valley P.T.A.", Jeannie C. Riley |
| Best Country Performance, Duo or Group Vocal or Instrumental |
"Foggy Mountain Breakdown", Flatt and Scruggs |
| Best Sacred Performance |
"Beautiful Isle of Somewhere", Jack Hess |
| Best Gospel Performance |
The Happy Gospel of the Happy Goodmans, Happy Goodman Family |
| Best Soul Gospel Performance |
"The Soul of Me", Dottie Rambo |
| Best Folk Performance |
"Both Sides Now", Judy Collins |
| Best Instrumental Arrangement |
"Classical Gas", Mike Post, arranger |
| Best Arrangement Accompanying Vocalist(s) |
"MacArthur Park", Jimmy L. Webb, arranger |
| Best Instrumental Theme |
"Classical Gas", Mason Williams, composer |
| Best Score From an Original Cast Show Album |
Hair, Gerome Ragni, James Rado and Galt MacDermott, composers (RCA) |
| Best Original Score Written for a Motion Picture or a Television Special |
The Graduate, Paul Simon and Dave Grusin, composers |
| Best Classical Performance, Orchestra |
Boulez Conducts Debussy, Pierre Boulez conducting New Philharmonia Orchestra |
| Best Chamber Music Performance |
Gabrieli, Canzoni for Brass, Winds, Strings and Organ, E. Power Biggs with Edward Tarr Ensemble and Gabrieli Consort; Vittorio Negri, conductor |
| Best Classical Performance, Instrumental Soloist(s) (With or Without Orchestra) |
Horowitz on Television, Vladimir Horowitz |
| Best Opera Recording |
Mozart, Cosi fan tutte, Erich Leinsdorf conducting New Philharmonia Orchestra and Ambrosian Opera Chorus; solos: Price, Raskin, Troyanos, Milnes, Shirley and Flagello (RCA) |
| Best Choral Performance (Other Than Opera) |
The Glory of Gabrieli, Vittorio Negri conducting Gregg Smith Singers and Texas Boys Choir; George Bragg directing Edward Tarr Ensemble with E. Power Biggs |
| Best Classical Vocal Soloist Performance |
Rossini Rarities, Montserrat Caballe; Carlo Felice Cillario conducting RCA Italiana Opera Orchestra and Chorus |
| Best Comedy Recording |
To Russell, My Brother, Whom I Slept With, Bill Cosby (Warner Bros.) |
| Best Spoken Word Recording |
Lonesome Cities, Rod McKuen (Warner Bros.-Seven Arts) |
| Best Album Cover |
Underground, John Berg and Richard Mantel, art directors (Columbia) |
| Best Album Notes |
Johnny Cash at Folsom Prison, Johnny Cash, annotator |